TY - JOUR
T1 - A simple and universal strategy to deposit Ag/polypyrrole on various substrates for enhanced interfacial solar evaporation and antibacterial activity
AU - Xu, Ying
AU - Ma, Jiaxiang
AU - Han, Yu
AU - Xu, Hongbo
AU - Wang, Yu
AU - Qi, Dianpeng
AU - Wang, Wei
N1 - Generated from Scopus record by KAUST IRTS on 2023-09-21
PY - 2020/3/15
Y1 - 2020/3/15
N2 - Solar-driven distillation is now considered as a rising technology for the supply of fresh water in the rare areas. As the crucial part of solar distillation, photothermal materials have been flourished investigated. Herein, we report a universal and facile method to construct a photothermal layer on various substrates to enhance the interfacial water evaporation via polypyrrole (PPy) polymerization and silver nanoparticles (Ag NPs) deposition. The photothermal Ag/PPy layer was firmly coated on six different substrates with an average solar absorption of 95.4% and Ag loading of 94.3 mg/L. One of the optimized resultant membranes (substrate is cellulose fibers) presents the ultrahigh solar evaporation rate of 1.55 kg m−2h−1 and a corresponding light-to-vapor efficiency of 92.6% with a silver loading of 74 μg cm−2. Bacterial diffusion inhibition zone experiments revealed clear antibacterial effects of the Ag/PPy membrane on bacteria. Furthermore, the Ag NPs deposited membrane had a rechargeability for multiple times upon their depletion, indicating sustainable anti-bacteria potential. Hence, our facial fabricated photothermal Ag/PPy layer can apply to substrates with different types for enhanced photothermal and anti-biocorrosion capacity, and may pave a new way to the long-term practical sustainable technique for the clean water production application.
AB - Solar-driven distillation is now considered as a rising technology for the supply of fresh water in the rare areas. As the crucial part of solar distillation, photothermal materials have been flourished investigated. Herein, we report a universal and facile method to construct a photothermal layer on various substrates to enhance the interfacial water evaporation via polypyrrole (PPy) polymerization and silver nanoparticles (Ag NPs) deposition. The photothermal Ag/PPy layer was firmly coated on six different substrates with an average solar absorption of 95.4% and Ag loading of 94.3 mg/L. One of the optimized resultant membranes (substrate is cellulose fibers) presents the ultrahigh solar evaporation rate of 1.55 kg m−2h−1 and a corresponding light-to-vapor efficiency of 92.6% with a silver loading of 74 μg cm−2. Bacterial diffusion inhibition zone experiments revealed clear antibacterial effects of the Ag/PPy membrane on bacteria. Furthermore, the Ag NPs deposited membrane had a rechargeability for multiple times upon their depletion, indicating sustainable anti-bacteria potential. Hence, our facial fabricated photothermal Ag/PPy layer can apply to substrates with different types for enhanced photothermal and anti-biocorrosion capacity, and may pave a new way to the long-term practical sustainable technique for the clean water production application.
UR - https://linkinghub.elsevier.com/retrieve/pii/S1385894719327925
UR - http://www.scopus.com/inward/record.url?scp=85075369388&partnerID=8YFLogxK
U2 - 10.1016/j.cej.2019.123379
DO - 10.1016/j.cej.2019.123379
M3 - Article
SN - 1385-8947
VL - 384
JO - Chemical Engineering Journal
JF - Chemical Engineering Journal
ER -