TY - JOUR
T1 - An Easy-to-Fabricate 2.5D Evaporator for Efficient Solar Desalination
AU - Liu, Xiaojie
AU - Tian, Yanpei
AU - Chen, Fangqi
AU - Caratenuto, Andrew
AU - DeGiorgis, Joseph A.
AU - ELSonbaty, Mohamed
AU - Wan, Yinsheng
AU - Ahlgren, Ralph
AU - Zheng, Yi
N1 - Generated from Scopus record by KAUST IRTS on 2023-09-23
PY - 2021/7/1
Y1 - 2021/7/1
N2 - Solar-driven steam generation, whereby solar energy is harvested to purify water directly, is emerging as a promising approach to mitigate the worldwide water crisis. The scalable application of conventional 3D evaporators is hindered by their complex spatial geometries. A 2.5D structure is a spatial extension of a 2D structure with an addition of a third vertical dimension, achieving both the feasibility of 2D structure and the performance of 3D structure simultaneously. Here, an interconnected open-pore 2.5D Cu/CuO foam-based photothermal evaporator capable of achieving a high evaporation rate of 4.1 kg m−2 h−1 under one sun illumination by exposing one end of the planar structure to air is demonstrated. The micro-sized open-pore structure of Cu/CuO foam allows it to trap incident sunlight, and the densely distributed blade-like CuO nanostructures effectively scatter sunlight inside pores simultaneously. The inherent hydrophilicity of CuO and capillarity forces from the porous structure of Cu foam continuously supply sufficient water. Moreover, the doubled working sides of Cu/CuO foam enlarge the exposure area enabling efficient vapor diffusion. The feasible fabrication process and the combined structural features of Cu/CuO foam offer new insight into the future development of solar-driven evaporators in large-scale applications with practical durability.
AB - Solar-driven steam generation, whereby solar energy is harvested to purify water directly, is emerging as a promising approach to mitigate the worldwide water crisis. The scalable application of conventional 3D evaporators is hindered by their complex spatial geometries. A 2.5D structure is a spatial extension of a 2D structure with an addition of a third vertical dimension, achieving both the feasibility of 2D structure and the performance of 3D structure simultaneously. Here, an interconnected open-pore 2.5D Cu/CuO foam-based photothermal evaporator capable of achieving a high evaporation rate of 4.1 kg m−2 h−1 under one sun illumination by exposing one end of the planar structure to air is demonstrated. The micro-sized open-pore structure of Cu/CuO foam allows it to trap incident sunlight, and the densely distributed blade-like CuO nanostructures effectively scatter sunlight inside pores simultaneously. The inherent hydrophilicity of CuO and capillarity forces from the porous structure of Cu foam continuously supply sufficient water. Moreover, the doubled working sides of Cu/CuO foam enlarge the exposure area enabling efficient vapor diffusion. The feasible fabrication process and the combined structural features of Cu/CuO foam offer new insight into the future development of solar-driven evaporators in large-scale applications with practical durability.
UR - https://onlinelibrary.wiley.com/doi/10.1002/adfm.202100911
UR - http://www.scopus.com/inward/record.url?scp=85104788466&partnerID=8YFLogxK
U2 - 10.1002/adfm.202100911
DO - 10.1002/adfm.202100911
M3 - Article
SN - 1057-9257
VL - 31
JO - Advanced Functional Materials
JF - Advanced Functional Materials
IS - 27
ER -