Catalytic ozonation with metal oxides: An option to control THM formation potential

T. Zhang; J. Ma; J. Lu; Z. Chen; C. Li; J. Jiang

doi:10.2166/ws.2006.760

Catalytic ozonation with metal oxides: An option to control THM formation potential

T. Zhang^*, J. Ma, J. Lu, Z. Chen, C. Li, J. Jiang

^*Corresponding author for this work

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

7 Scopus citations

Abstract

This paper aimed at illustrating the impact of catalytic ozonation on trihalomethane formation potential (THMsFP) of a filtered surface water. Catalytic ozonation with several metal oxides (synthetic α-FeOOH (FeOOH), γ·Al₂O₃ (Al₂O₃), CeO₂ and MgO) significantly reduced THMsFP of the water compared with ozonation alone. For the FeOOH catalyzed ozonation, several factors, including bromide concentration, pH, alkalinity, ozone dosage, and reaction time, were further studied for their effect on THMsFP of the water. The FeOOH/O₃ showed a significant advantage over ozonation in controlling the THMsFP at the applied conditions of bromide (0-3.36 mg/L), pH (6.33-9.43), O₃/DOC ratio (0.65-2.05 mg/mg), and reaction time (2-20 min). Increase of bicarbonate alkalinity weakened its advantage. The possible mechanism for the FeOOH/O ₃ in controlling the THMsFP can be ascribed to higher DOC removal rate and enhanced oxidation of some precursors.

Original language	English (US)
Title of host publication	5th World Water Congress
Subtitle of host publication	Drinking Water Treatment Processes
Editors	G. Amy, Ajit Annachhatre, Erik Arvin, Jining Chen, Jaewon Cho
Pages	63-70
Number of pages	8
Edition	3
DOIs	https://doi.org/10.2166/ws.2006.760
State	Published - 2006
Externally published	Yes

Publication series

Name	Water Science and Technology: Water Supply
Number	3
Volume	6
ISSN (Print)	1606-9749

Keywords

Bromide
Catalytic ozonation
FeOOH
Filtered water
Metal oxides
THMsFP

ASJC Scopus subject areas

Water Science and Technology

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10.2166/ws.2006.760

Cite this

Zhang, T., Ma, J., Lu, J., Chen, Z., Li, C., & Jiang, J. (2006). Catalytic ozonation with metal oxides: An option to control THM formation potential. In G. Amy, A. Annachhatre, E. Arvin, J. Chen, & J. Cho (Eds.), 5th World Water Congress: Drinking Water Treatment Processes (3 ed., pp. 63-70). (Water Science and Technology: Water Supply; Vol. 6, No. 3). https://doi.org/10.2166/ws.2006.760

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title = "Catalytic ozonation with metal oxides: An option to control THM formation potential",

abstract = "This paper aimed at illustrating the impact of catalytic ozonation on trihalomethane formation potential (THMsFP) of a filtered surface water. Catalytic ozonation with several metal oxides (synthetic α-FeOOH (FeOOH), γ·Al2O3 (Al2O3), CeO2 and MgO) significantly reduced THMsFP of the water compared with ozonation alone. For the FeOOH catalyzed ozonation, several factors, including bromide concentration, pH, alkalinity, ozone dosage, and reaction time, were further studied for their effect on THMsFP of the water. The FeOOH/O3 showed a significant advantage over ozonation in controlling the THMsFP at the applied conditions of bromide (0-3.36 mg/L), pH (6.33-9.43), O3/DOC ratio (0.65-2.05 mg/mg), and reaction time (2-20 min). Increase of bicarbonate alkalinity weakened its advantage. The possible mechanism for the FeOOH/O 3 in controlling the THMsFP can be ascribed to higher DOC removal rate and enhanced oxidation of some precursors.",

keywords = "Bromide, Catalytic ozonation, FeOOH, Filtered water, Metal oxides, THMsFP",

author = "T. Zhang and J. Ma and J. Lu and Z. Chen and C. Li and J. Jiang",

year = "2006",

doi = "10.2166/ws.2006.760",

language = "English (US)",

isbn = "1843395878",

series = "Water Science and Technology: Water Supply",

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}

Zhang, T, Ma, J, Lu, J, Chen, Z, Li, C & Jiang, J 2006, Catalytic ozonation with metal oxides: An option to control THM formation potential. in G Amy, A Annachhatre, E Arvin, J Chen & J Cho (eds), 5th World Water Congress: Drinking Water Treatment Processes. 3 edn, Water Science and Technology: Water Supply, no. 3, vol. 6, pp. 63-70. https://doi.org/10.2166/ws.2006.760

Catalytic ozonation with metal oxides: An option to control THM formation potential. / Zhang, T.; Ma, J.; Lu, J. et al.
5th World Water Congress: Drinking Water Treatment Processes. ed. / G. Amy; Ajit Annachhatre; Erik Arvin; Jining Chen; Jaewon Cho. 3. ed. 2006. p. 63-70 (Water Science and Technology: Water Supply; Vol. 6, No. 3).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

TY - GEN

T1 - Catalytic ozonation with metal oxides

T2 - An option to control THM formation potential

AU - Zhang, T.

AU - Ma, J.

AU - Lu, J.

AU - Chen, Z.

AU - Li, C.

AU - Jiang, J.

PY - 2006

Y1 - 2006

N2 - This paper aimed at illustrating the impact of catalytic ozonation on trihalomethane formation potential (THMsFP) of a filtered surface water. Catalytic ozonation with several metal oxides (synthetic α-FeOOH (FeOOH), γ·Al2O3 (Al2O3), CeO2 and MgO) significantly reduced THMsFP of the water compared with ozonation alone. For the FeOOH catalyzed ozonation, several factors, including bromide concentration, pH, alkalinity, ozone dosage, and reaction time, were further studied for their effect on THMsFP of the water. The FeOOH/O3 showed a significant advantage over ozonation in controlling the THMsFP at the applied conditions of bromide (0-3.36 mg/L), pH (6.33-9.43), O3/DOC ratio (0.65-2.05 mg/mg), and reaction time (2-20 min). Increase of bicarbonate alkalinity weakened its advantage. The possible mechanism for the FeOOH/O 3 in controlling the THMsFP can be ascribed to higher DOC removal rate and enhanced oxidation of some precursors.

AB - This paper aimed at illustrating the impact of catalytic ozonation on trihalomethane formation potential (THMsFP) of a filtered surface water. Catalytic ozonation with several metal oxides (synthetic α-FeOOH (FeOOH), γ·Al2O3 (Al2O3), CeO2 and MgO) significantly reduced THMsFP of the water compared with ozonation alone. For the FeOOH catalyzed ozonation, several factors, including bromide concentration, pH, alkalinity, ozone dosage, and reaction time, were further studied for their effect on THMsFP of the water. The FeOOH/O3 showed a significant advantage over ozonation in controlling the THMsFP at the applied conditions of bromide (0-3.36 mg/L), pH (6.33-9.43), O3/DOC ratio (0.65-2.05 mg/mg), and reaction time (2-20 min). Increase of bicarbonate alkalinity weakened its advantage. The possible mechanism for the FeOOH/O 3 in controlling the THMsFP can be ascribed to higher DOC removal rate and enhanced oxidation of some precursors.

KW - Bromide

KW - Catalytic ozonation

KW - FeOOH

KW - Filtered water

KW - Metal oxides

KW - THMsFP

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DO - 10.2166/ws.2006.760

M3 - Conference contribution

AN - SCOPUS:33845235994

SN - 1843395878

SN - 9781843395874

T3 - Water Science and Technology: Water Supply

SP - 63

EP - 70

BT - 5th World Water Congress

A2 - Amy, G.

A2 - Annachhatre, Ajit

A2 - Arvin, Erik

A2 - Chen, Jining

A2 - Cho, Jaewon

ER -

Catalytic ozonation with metal oxides: An option to control THM formation potential

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