Electrically switchable anisotropic polariton propagation in a ferroelectric van der Waals semiconductor.

Yue Luo, Nannan Mao, Dapeng Ding, Ming-Hui Chiu, Xiang Ji, Kenji Watanabe, Takashi Taniguchi, Vincent Tung, Hongkun Park, Philip Kim, Jing Kong, William L Wilson

Research output: Contribution to journalArticlepeer-review

13 Scopus citations

Abstract

Tailoring of the propagation dynamics of exciton-polaritons in two-dimensional quantum materials has shown extraordinary promise to enable nanoscale control of electromagnetic fields. Varying permittivities along crystal directions within layers of material systems, can lead to an in-plane anisotropic dispersion of polaritons. Exploiting this physics as a control strategy for manipulating the directional propagation of the polaritons is desired and remains elusive. Here we explore the in-plane anisotropic exciton-polariton propagation in SnSe, a group-IV monochalcogenide semiconductor that forms ferroelectric domains and shows room-temperature excitonic behaviour. Exciton-polaritons are launched in SnSe multilayer plates, and their propagation dynamics and dispersion are studied. This propagation of exciton-polaritons allows for nanoscale imaging of the in-plane ferroelectric domains. Finally, we demonstrate the electric switching of the exciton-polaritons in the ferroelectric domains of this complex van der Waals system. The study suggests that systems such as group-IV monochalcogenides could serve as excellent ferroic platforms for actively reconfigurable polaritonic optical devices.
Original languageEnglish (US)
JournalNature Nanotechnology
DOIs
StatePublished - Jan 23 2023

ASJC Scopus subject areas

  • Biomedical Engineering
  • Bioengineering
  • General Materials Science
  • Atomic and Molecular Physics, and Optics
  • Electrical and Electronic Engineering
  • Condensed Matter Physics

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