TY - JOUR
T1 - Fully analytical description of adiabatic compression in dissipative polaritonic structures
AU - Proietti Zaccaria, Remo
AU - Alabastri, Alessandro
AU - De Angelis, Francesco
AU - Das, Gobind
AU - Liberale, Carlo
AU - Toma, Andrea
AU - Giugni, Andrea
AU - Razzari, Luca
AU - Malerba, Mario
AU - Sun, Hong Bo
AU - Di Fabrizio, Enzo
PY - 2012/7/5
Y1 - 2012/7/5
N2 - We have theoretically modeled and experimentally fabricated a nanoscale adiabatic (conical) metallic structure that is suitable for high-resolution Raman spectroscopy. We report on a fully complex analytical description of the adiabatic compression phenomenon which is investigated in terms of both geometrical and optical parameters. An explicit analytical description of adiabatic compression is provided together with the physical role played by the complex effective refractive index of the polaritonic adiabatic mode. In particular, we have examined the role of absorption on the field enhancement. Finally, we demonstrate how such a device can experimentally enhance the Raman signal coming from nanosamples such as a bead of SiO x and a monolayer of benzenethiol.
AB - We have theoretically modeled and experimentally fabricated a nanoscale adiabatic (conical) metallic structure that is suitable for high-resolution Raman spectroscopy. We report on a fully complex analytical description of the adiabatic compression phenomenon which is investigated in terms of both geometrical and optical parameters. An explicit analytical description of adiabatic compression is provided together with the physical role played by the complex effective refractive index of the polaritonic adiabatic mode. In particular, we have examined the role of absorption on the field enhancement. Finally, we demonstrate how such a device can experimentally enhance the Raman signal coming from nanosamples such as a bead of SiO x and a monolayer of benzenethiol.
UR - http://www.scopus.com/inward/record.url?scp=84863703220&partnerID=8YFLogxK
U2 - 10.1103/PhysRevB.86.035410
DO - 10.1103/PhysRevB.86.035410
M3 - Article
AN - SCOPUS:84863703220
SN - 1098-0121
VL - 86
JO - Physical Review B - Condensed Matter and Materials Physics
JF - Physical Review B - Condensed Matter and Materials Physics
IS - 3
M1 - 035410
ER -