TY - JOUR
T1 - Harnessing structural darkness in the visible and infrared wavelengths for a new source of light
AU - Huang, Jianfeng
AU - Liu, Changxu
AU - Zhu, Yihan
AU - Masala, Silvia
AU - Alarousu, Erkki
AU - Han, Yu
AU - Fratalocchi, Andrea
N1 - KAUST Repository Item: Exported on 2020-10-01
Acknowledgements: This work is part of the Kaust research programme 'Optics and plasmonics for efficient energy harvesting', supported by award no. CRG-1-2012-FRA-005. Y.H. acknowledges baseline support funds from Kaust.
PY - 2015/10/19
Y1 - 2015/10/19
N2 - Engineering broadband light absorbers is crucial to many applications, including energy-harvesting devices and optical interconnects. The performances of an ideal absorber are that of a black body, a dark material that absorbs radiation at all angles and polarizations. Despite advances in micrometre-thick films, the absorbers available to date are still far from an ideal black body. Here, we describe a disordered nanostructured material that shows an almost ideal black-body absorption of 98-99% between 400 and 1,400 nm that is insensitive to the angle and polarization of the incident light. The material comprises nanoparticles composed of a nanorod with a nanosphere of 30 nm diameter attached. When diluted into liquids, a small concentration of nanoparticles absorbs on average 26% more than carbon nanotubes, the darkest material available to date. By pumping a dye optical amplifier with nanosecond pulses of 100 mW power, we harness the structural darkness of the material and create a new type of light source, which generates monochromatic emission (5 nm wide) without the need for any resonance. This is achieved through the dynamics of light condensation in which all absorbed electromagnetic energy spontaneously generates single-colour energy pulses. © 2016 Macmillan Publishers Limited. All rights reserved.
AB - Engineering broadband light absorbers is crucial to many applications, including energy-harvesting devices and optical interconnects. The performances of an ideal absorber are that of a black body, a dark material that absorbs radiation at all angles and polarizations. Despite advances in micrometre-thick films, the absorbers available to date are still far from an ideal black body. Here, we describe a disordered nanostructured material that shows an almost ideal black-body absorption of 98-99% between 400 and 1,400 nm that is insensitive to the angle and polarization of the incident light. The material comprises nanoparticles composed of a nanorod with a nanosphere of 30 nm diameter attached. When diluted into liquids, a small concentration of nanoparticles absorbs on average 26% more than carbon nanotubes, the darkest material available to date. By pumping a dye optical amplifier with nanosecond pulses of 100 mW power, we harness the structural darkness of the material and create a new type of light source, which generates monochromatic emission (5 nm wide) without the need for any resonance. This is achieved through the dynamics of light condensation in which all absorbed electromagnetic energy spontaneously generates single-colour energy pulses. © 2016 Macmillan Publishers Limited. All rights reserved.
UR - http://hdl.handle.net/10754/621595
UR - http://www.nature.com/articles/nnano.2015.228
UR - http://www.scopus.com/inward/record.url?scp=84954379239&partnerID=8YFLogxK
U2 - 10.1038/nnano.2015.228
DO - 10.1038/nnano.2015.228
M3 - Article
C2 - 26479025
SN - 1748-3387
VL - 11
SP - 60
EP - 66
JO - Nature Nanotechnology
JF - Nature Nanotechnology
IS - 1
ER -