TY - JOUR
T1 - Ligand-controlled stereodivergent alkenylation of alkynes to access functionalized trans- and cis-1,3-dienes
AU - Long, Tianyu
AU - Zhu, Chen
AU - Li, Ling
AU - Shao, Liang
AU - Zhu, Shengqing
AU - Rueping, Magnus
AU - Chu, Lingling
N1 - KAUST Repository Item: Exported on 2023-01-06
Acknowledged KAUST grant number(s): URF/1/4025
Acknowledgements: The authors are grateful for the financial support provided by the National Natural Science Foundation of China (21971036), the National Science Fund for Excellent Young Scholars (22122101), the Shanghai Rising-Star Program (20QA1400200), the King Abdullah University of Science and Technology (KAUST), Saudi Arabia, Office of Sponsored Research (URF/1/4025). The authors acknowledge the KAUST Supercomputing Laboratory for providing the computational resources of the Shaheen-II supercomputer.
PY - 2023/1/4
Y1 - 2023/1/4
N2 - Precise stereocontrol of functionalized alkenes represents a long-standing research topic in organic synthesis. Nevertheless, the development of a catalytic, easily tunable synthetic approach for the stereodivergent synthesis of both E-selective and even more challenging Z-selective highly substituted 1,3-dienes from common substrates remains underexploited. Here, we report a photoredox and nickel dual catalytic strategy for the stereodivergent sulfonylalkenylation of terminal alkynes with vinyl triflates and sodium sulfinates under mild conditions. With a judicious choice of simple nickel catalyst and ligand, this method enables efficient and divergent access to both Z- and E-sulfonyl-1,3-dienes from the same set of simple starting materials. This method features broad substrate scope, good functional compatibility, and excellent chemo-, regio-, and stereoselectivity. Experimental and DFT mechanistic studies offer insights into the observed divergent stereoselectivity controlled by ligands.
AB - Precise stereocontrol of functionalized alkenes represents a long-standing research topic in organic synthesis. Nevertheless, the development of a catalytic, easily tunable synthetic approach for the stereodivergent synthesis of both E-selective and even more challenging Z-selective highly substituted 1,3-dienes from common substrates remains underexploited. Here, we report a photoredox and nickel dual catalytic strategy for the stereodivergent sulfonylalkenylation of terminal alkynes with vinyl triflates and sodium sulfinates under mild conditions. With a judicious choice of simple nickel catalyst and ligand, this method enables efficient and divergent access to both Z- and E-sulfonyl-1,3-dienes from the same set of simple starting materials. This method features broad substrate scope, good functional compatibility, and excellent chemo-, regio-, and stereoselectivity. Experimental and DFT mechanistic studies offer insights into the observed divergent stereoselectivity controlled by ligands.
UR - http://hdl.handle.net/10754/686800
UR - https://www.nature.com/articles/s41467-022-35688-2
U2 - 10.1038/s41467-022-35688-2
DO - 10.1038/s41467-022-35688-2
M3 - Article
C2 - 36599820
SN - 2041-1723
VL - 14
JO - Nature Communications
JF - Nature Communications
IS - 1
ER -