Mechanochemically-based three-way approach for the synthesis of K-doped Cu-Fe/ZnO-Al2O3 catalysts for converting CO2 to oxygenates

Boon Ying Tay; Charmain Kan; Jennet Ong; Shashikant U. Dighe; Amol M. Hengne; Kuo Wei Huang; Lili Zhang; Roong Jien Wong; Davin Tan

doi:10.1039/d4cc02073a

Mechanochemically-based three-way approach for the synthesis of K-doped Cu-Fe/ZnO-Al₂O₃ catalysts for converting CO₂ to oxygenates

Boon Ying Tay, Charmain Kan, Jennet Ong, Shashikant U. Dighe, Amol M. Hengne, Kuo Wei Huang, Lili Zhang, Roong Jien Wong^*, Davin Tan^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

Abstract

Three ball-milling methodologies were developed to synthesize bespoke multi-metallic K-doped Cu-Fe/ZnO-Al₂O₃ catalysts for the hydrogenation of carbon dioxide. The catalytic performance of the catalysts was benchmarked against their solution-based counterparts. The catalysts synthesized by ball milling are greener, showing smaller particles, with different selectivity towards oxygenate products.

Original language	English (US)
Pages (from-to)	10890-10893
Number of pages	4
Journal	CHEMICAL COMMUNICATIONS
Volume	60
Issue number	78
DOIs	https://doi.org/10.1039/d4cc02073a
State	Published - Sep 3 2024

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Catalysis
Ceramics and Composites
General Chemistry
Surfaces, Coatings and Films
Metals and Alloys
Materials Chemistry

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title = "Mechanochemically-based three-way approach for the synthesis of K-doped Cu-Fe/ZnO-Al2O3 catalysts for converting CO2 to oxygenates",

abstract = "Three ball-milling methodologies were developed to synthesize bespoke multi-metallic K-doped Cu-Fe/ZnO-Al2O3 catalysts for the hydrogenation of carbon dioxide. The catalytic performance of the catalysts was benchmarked against their solution-based counterparts. The catalysts synthesized by ball milling are greener, showing smaller particles, with different selectivity towards oxygenate products.",

author = "Tay, {Boon Ying} and Charmain Kan and Jennet Ong and Dighe, {Shashikant U.} and Hengne, {Amol M.} and Huang, {Kuo Wei} and Lili Zhang and Wong, {Roong Jien} and Davin Tan",

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doi = "10.1039/d4cc02073a",

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T1 - Mechanochemically-based three-way approach for the synthesis of K-doped Cu-Fe/ZnO-Al2O3 catalysts for converting CO2 to oxygenates

AU - Tay, Boon Ying

AU - Kan, Charmain

AU - Ong, Jennet

AU - Dighe, Shashikant U.

AU - Hengne, Amol M.

AU - Huang, Kuo Wei

AU - Zhang, Lili

AU - Wong, Roong Jien

AU - Tan, Davin

PY - 2024/9/3

Y1 - 2024/9/3

N2 - Three ball-milling methodologies were developed to synthesize bespoke multi-metallic K-doped Cu-Fe/ZnO-Al2O3 catalysts for the hydrogenation of carbon dioxide. The catalytic performance of the catalysts was benchmarked against their solution-based counterparts. The catalysts synthesized by ball milling are greener, showing smaller particles, with different selectivity towards oxygenate products.

AB - Three ball-milling methodologies were developed to synthesize bespoke multi-metallic K-doped Cu-Fe/ZnO-Al2O3 catalysts for the hydrogenation of carbon dioxide. The catalytic performance of the catalysts was benchmarked against their solution-based counterparts. The catalysts synthesized by ball milling are greener, showing smaller particles, with different selectivity towards oxygenate products.

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U2 - 10.1039/d4cc02073a

DO - 10.1039/d4cc02073a

M3 - Article

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AN - SCOPUS:85204176498

SN - 1359-7345

VL - 60

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JO - CHEMICAL COMMUNICATIONS

JF - CHEMICAL COMMUNICATIONS

IS - 78

ER -

Mechanochemically-based three-way approach for the synthesis of K-doped Cu-Fe/ZnO-Al₂O₃ catalysts for converting CO₂ to oxygenates

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