Modeling and parametric analysis of hollow fiber membrane system for carbon capture from multicomponent flue gas

Rajab Khalilpour; Ali Abbas; Zhiping Lai; Ingo Pinnau

doi:10.1002/aic.12699

Modeling and parametric analysis of hollow fiber membrane system for carbon capture from multicomponent flue gas

Rajab Khalilpour, Ali Abbas, Zhiping Lai, Ingo Pinnau

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34 Scopus citations

Abstract

The modeling and optimal design/operation of gas membranes for postcombustion carbon capture (PCC) is presented. A systematic methodology is presented for analysis of membrane systems considering multicomponent flue gas with CO 2 as target component. Simplifying assumptions is avoided by namely multicomponent flue gas represented by CO 2/N 2 binary mixture or considering the co/countercurrent flow pattern of hollow-fiber membrane system as mixed flow. Optimal regions of flue gas pressures and membrane area were found within which a technoeconomical process system design could be carried out. High selectivity was found to not necessarily have notable impact on PCC membrane performance, rather, a medium selectivity combined with medium or high permeance could be more advantageous. © 2011 American Institute of Chemical Engineers (AIChE).

Original language	English (US)
Pages (from-to)	1550-1561
Number of pages	12
Journal	AIChE Journal
Volume	58
Issue number	5
DOIs	https://doi.org/10.1002/aic.12699
State	Published - Aug 12 2011

ASJC Scopus subject areas

General Chemical Engineering
Biotechnology
Environmental Engineering

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abstract = "The modeling and optimal design/operation of gas membranes for postcombustion carbon capture (PCC) is presented. A systematic methodology is presented for analysis of membrane systems considering multicomponent flue gas with CO 2 as target component. Simplifying assumptions is avoided by namely multicomponent flue gas represented by CO 2/N 2 binary mixture or considering the co/countercurrent flow pattern of hollow-fiber membrane system as mixed flow. Optimal regions of flue gas pressures and membrane area were found within which a technoeconomical process system design could be carried out. High selectivity was found to not necessarily have notable impact on PCC membrane performance, rather, a medium selectivity combined with medium or high permeance could be more advantageous. {\textcopyright} 2011 American Institute of Chemical Engineers (AIChE).",

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AU - Khalilpour, Rajab

AU - Abbas, Ali

AU - Lai, Zhiping

AU - Pinnau, Ingo

N1 - KAUST Repository Item: Exported on 2020-10-01 Acknowledgements: The authors gratefully acknowledge Delta Electricity's sponsorship of this project.

PY - 2011/8/12

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Modeling and parametric analysis of hollow fiber membrane system for carbon capture from multicomponent flue gas

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