Non-oxidative coupling of methane catalysed by supported tungsten hydride onto alumina and silica-alumina in classical and H2 permeable membrane fixed-bed reactors

K. C. Szeto; S. Norsic; L. Hardou; E. Le Roux; S. Chakka; J. Thivolle-Cazat; A. Baudouin; C. Papaioannou; J. M. Basset; M. Taoufik

doi:10.1039/c0cc00007h

Non-oxidative coupling of methane catalysed by supported tungsten hydride onto alumina and silica-alumina in classical and H₂ permeable membrane fixed-bed reactors

K. C. Szeto, S. Norsic, L. Hardou, E. Le Roux, S. Chakka, J. Thivolle-Cazat, A. Baudouin, C. Papaioannou, J. M. Basset^*, M. Taoufik

^*Corresponding author for this work

Physical Sciences and Engineering

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36 Scopus citations

Abstract

Non-oxidative coupling of methane with high selectivity into ethane (>99% among hydrocarbon) in a classical fixed-bed reactor catalysed by SiO₂-Al₂O₃ or γ-Al₂O ₃ supported tungsten hydride is presented. Continuous hydrogen separation, using a Pd-Ag membrane in a fixed-bed reactor, led to methane coupling far beyond the thermodynamic equilibrium conversion.

Original language	English (US)
Pages (from-to)	3985-3987
Number of pages	3
Journal	CHEMICAL COMMUNICATIONS
Volume	46
Issue number	22
DOIs	https://doi.org/10.1039/c0cc00007h
State	Published - Jun 14 2010

ASJC Scopus subject areas

Catalysis
Electronic, Optical and Magnetic Materials
Ceramics and Composites
General Chemistry
Surfaces, Coatings and Films
Metals and Alloys
Materials Chemistry

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Szeto, K. C., Norsic, S., Hardou, L., Le Roux, E., Chakka, S., Thivolle-Cazat, J., Baudouin, A., Papaioannou, C., Basset, J. M., & Taoufik, M. (2010). Non-oxidative coupling of methane catalysed by supported tungsten hydride onto alumina and silica-alumina in classical and H₂ permeable membrane fixed-bed reactors. CHEMICAL COMMUNICATIONS, 46(22), 3985-3987. https://doi.org/10.1039/c0cc00007h

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abstract = "Non-oxidative coupling of methane with high selectivity into ethane (>99% among hydrocarbon) in a classical fixed-bed reactor catalysed by SiO2-Al2O3 or γ-Al2O 3 supported tungsten hydride is presented. Continuous hydrogen separation, using a Pd-Ag membrane in a fixed-bed reactor, led to methane coupling far beyond the thermodynamic equilibrium conversion.",

author = "Szeto, {K. C.} and S. Norsic and L. Hardou and {Le Roux}, E. and S. Chakka and J. Thivolle-Cazat and A. Baudouin and C. Papaioannou and Basset, {J. M.} and M. Taoufik",

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doi = "10.1039/c0cc00007h",

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Szeto, KC, Norsic, S, Hardou, L, Le Roux, E, Chakka, S, Thivolle-Cazat, J, Baudouin, A, Papaioannou, C, Basset, JM & Taoufik, M 2010, 'Non-oxidative coupling of methane catalysed by supported tungsten hydride onto alumina and silica-alumina in classical and H₂ permeable membrane fixed-bed reactors', CHEMICAL COMMUNICATIONS, vol. 46, no. 22, pp. 3985-3987. https://doi.org/10.1039/c0cc00007h

TY - JOUR

T1 - Non-oxidative coupling of methane catalysed by supported tungsten hydride onto alumina and silica-alumina in classical and H2 permeable membrane fixed-bed reactors

AU - Szeto, K. C.

AU - Norsic, S.

AU - Hardou, L.

AU - Le Roux, E.

AU - Chakka, S.

AU - Thivolle-Cazat, J.

AU - Baudouin, A.

AU - Papaioannou, C.

AU - Basset, J. M.

AU - Taoufik, M.

PY - 2010/6/14

Y1 - 2010/6/14

N2 - Non-oxidative coupling of methane with high selectivity into ethane (>99% among hydrocarbon) in a classical fixed-bed reactor catalysed by SiO2-Al2O3 or γ-Al2O 3 supported tungsten hydride is presented. Continuous hydrogen separation, using a Pd-Ag membrane in a fixed-bed reactor, led to methane coupling far beyond the thermodynamic equilibrium conversion.

AB - Non-oxidative coupling of methane with high selectivity into ethane (>99% among hydrocarbon) in a classical fixed-bed reactor catalysed by SiO2-Al2O3 or γ-Al2O 3 supported tungsten hydride is presented. Continuous hydrogen separation, using a Pd-Ag membrane in a fixed-bed reactor, led to methane coupling far beyond the thermodynamic equilibrium conversion.

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U2 - 10.1039/c0cc00007h

DO - 10.1039/c0cc00007h

M3 - Article

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AN - SCOPUS:77952774101

SN - 1359-7345

VL - 46

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EP - 3987

JO - CHEMICAL COMMUNICATIONS

JF - CHEMICAL COMMUNICATIONS

IS - 22

ER -

Non-oxidative coupling of methane catalysed by supported tungsten hydride onto alumina and silica-alumina in classical and H₂ permeable membrane fixed-bed reactors

Abstract

ASJC Scopus subject areas

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