State of the Art and Prospects for Halide Perovskite Nanocrystals

Amrita Dey; Junzhi Ye; Apurba De; Elke Debroye; Seung Kyun Ha; Eva Bladt; Anuraj S. Kshirsagar; Ziyu Wang; Jun Yin; Yue Wang; Li Na Quan; Fei Yan; Mengyu Gao; Xiaoming Li; Javad Shamsi; Tushar Debnath; Muhan Cao; Manuel A. Scheel; Sudhir Kumar; Julian A. Steele; Marina Gerhard; Lata Chouhan; Ke Xu; Xian-gang Wu; Yanxiu Li; Yangning Zhang; Anirban Dutta; Chuang Han; Ilka Vincon; Andrey L. Rogach; Angshuman Nag; Anunay Samanta; Brian A. Korgel; Chih-Jen Shih; Daniel R. Gamelin; Dong Hee Son; Haibo Zeng; Haizheng Zhong; Handong Sun; Hilmi Volkan Demir; Ivan G. Scheblykin; Iván Mora-Seró; Jacek K. Stolarczyk; Jin Z. Zhang; Jochen Feldmann; Johan Hofkens; Joseph Luther; Julia Pérez-Prieto; Liang Li; Liberato Manna; Maryna I. Bodnarchuk; Maksym V. Kovalenko; Maarten B. J. Roeffaers; Narayan Pradhan; Omar F. Mohammed; Osman Bakr; Peidong Yang; Peter Müller-Buschbaum; Prashant V. Kamat; Qialiang Bao; Qiao Zhang; Roman Krahne; Raquel E. Galian; Samuel D. Stranks; Sara Bals; Vasudevanpillai Biju; William A. Tisdale; Yong Yan; Robert L. Z. Hoye; Lakshminarayana Polavarapu

doi:10.1021/acsnano.0c08903

State of the Art and Prospects for Halide Perovskite Nanocrystals

Amrita Dey, Junzhi Ye, Apurba De, Elke Debroye, Seung Kyun Ha, Eva Bladt, Anuraj S. Kshirsagar, Ziyu Wang, Jun Yin, Yue Wang, Li Na Quan, Fei Yan, Mengyu Gao, Xiaoming Li, Javad Shamsi, Tushar Debnath, Muhan Cao, Manuel A. Scheel, Sudhir Kumar, Julian A. SteeleMarina Gerhard, Lata Chouhan, Ke Xu, Xian-gang Wu, Yanxiu Li, Yangning Zhang, Anirban Dutta, Chuang Han, Ilka Vincon, Andrey L. Rogach, Angshuman Nag, Anunay Samanta, Brian A. Korgel, Chih-Jen Shih, Daniel R. Gamelin, Dong Hee Son, Haibo Zeng, Haizheng Zhong, Handong Sun, Hilmi Volkan Demir, Ivan G. Scheblykin, Iván Mora-Seró, Jacek K. Stolarczyk, Jin Z. Zhang, Jochen Feldmann, Johan Hofkens, Joseph Luther, Julia Pérez-Prieto, Liang Li, Liberato Manna, Maryna I. Bodnarchuk, Maksym V. Kovalenko, Maarten B. J. Roeffaers, Narayan Pradhan, Omar F. Mohammed, Osman Bakr, Peidong Yang, Peter Müller-Buschbaum, Prashant V. Kamat, Qialiang Bao, Qiao Zhang, Roman Krahne, Raquel E. Galian, Samuel D. Stranks, Sara Bals, Vasudevanpillai Biju, William A. Tisdale, Yong Yan, Robert L. Z. Hoye, Lakshminarayana Polavarapu

Research output: Contribution to journal › Article › peer-review

819 Scopus citations

Abstract

Metal-halide perovskites have rapidly emerged as one of the most promising materials of the 21st century, with many exciting properties and great potential for a broad range of applications, from photovoltaics to optoelectronics and photocatalysis. The ease with which metal-halide perovskites can be synthesized in the form of brightly luminescent colloidal nanocrystals, as well as their tunable and intriguing optical and electronic properties, has attracted researchers from different disciplines of science and technology. In the last few years, there has been a significant progress in the shape-controlled synthesis of perovskite nanocrystals and understanding of their properties and applications. In this comprehensive review, researchers having expertise in different fields (chemistry, physics, and device engineering) of metal-halide perovskite nanocrystals have joined together to provide a state of the art overview and future prospects of metal-halide perovskite nanocrystal research.

Original language	English (US)
Journal	ACS Nano
DOIs	https://doi.org/10.1021/acsnano.0c08903
State	Published - Jun 17 2021

ASJC Scopus subject areas

General Physics and Astronomy
General Materials Science
General Engineering

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10.1021/acsnano.0c08903

Cite this

@article{c5ecaea412954fb882c60e33edb9804a,

title = "State of the Art and Prospects for Halide Perovskite Nanocrystals",

abstract = "Metal-halide perovskites have rapidly emerged as one of the most promising materials of the 21st century, with many exciting properties and great potential for a broad range of applications, from photovoltaics to optoelectronics and photocatalysis. The ease with which metal-halide perovskites can be synthesized in the form of brightly luminescent colloidal nanocrystals, as well as their tunable and intriguing optical and electronic properties, has attracted researchers from different disciplines of science and technology. In the last few years, there has been a significant progress in the shape-controlled synthesis of perovskite nanocrystals and understanding of their properties and applications. In this comprehensive review, researchers having expertise in different fields (chemistry, physics, and device engineering) of metal-halide perovskite nanocrystals have joined together to provide a state of the art overview and future prospects of metal-halide perovskite nanocrystal research.",

author = "Amrita Dey and Junzhi Ye and Apurba De and Elke Debroye and Ha, {Seung Kyun} and Eva Bladt and Kshirsagar, {Anuraj S.} and Ziyu Wang and Jun Yin and Yue Wang and Quan, {Li Na} and Fei Yan and Mengyu Gao and Xiaoming Li and Javad Shamsi and Tushar Debnath and Muhan Cao and Scheel, {Manuel A.} and Sudhir Kumar and Steele, {Julian A.} and Marina Gerhard and Lata Chouhan and Ke Xu and Xian-gang Wu and Yanxiu Li and Yangning Zhang and Anirban Dutta and Chuang Han and Ilka Vincon and Rogach, {Andrey L.} and Angshuman Nag and Anunay Samanta and Korgel, {Brian A.} and Chih-Jen Shih and Gamelin, {Daniel R.} and Son, {Dong Hee} and Haibo Zeng and Haizheng Zhong and Handong Sun and Demir, {Hilmi Volkan} and Scheblykin, {Ivan G.} and Iv{\'a}n Mora-Ser{\'o} and Stolarczyk, {Jacek K.} and Zhang, {Jin Z.} and Jochen Feldmann and Johan Hofkens and Joseph Luther and Julia P{\'e}rez-Prieto and Liang Li and Liberato Manna and Bodnarchuk, {Maryna I.} and Kovalenko, {Maksym V.} and Roeffaers, {Maarten B. J.} and Narayan Pradhan and Mohammed, {Omar F.} and Osman Bakr and Peidong Yang and Peter M{\"u}ller-Buschbaum and Kamat, {Prashant V.} and Qialiang Bao and Qiao Zhang and Roman Krahne and Galian, {Raquel E.} and Stranks, {Samuel D.} and Sara Bals and Vasudevanpillai Biju and Tisdale, {William A.} and Yong Yan and Hoye, {Robert L. Z.} and Lakshminarayana Polavarapu",

note = "KAUST Repository Item: Exported on 2021-06-22 Acknowledgements: L.P. acknowledges support from the Spanish Ministerio de Ciencia e Innovaci{\'o}n through Ram{\'o}n y Cajal grant (RYC2018-026103-I). A.D., T.D., I.V., J.K.S., J.F., M.A.S., P.M.-B. and L.P acknowledge financial support by the Bavarian State Ministry of Science, Research, and Arts through the grant “Solar Technologies go Hybrid (SolTech)” and by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany{\textquoteright}s Excellence Strategy—EXC 2089/1—390776260 (“e-conversion”). J.F., L.P., and V.D acknowledge support by LMU{\textquoteright}s “Singapore Initiative” funded within the German Excellence Strategy. H. Zeng acknowledges the support of NSFC (61874054, 51902160), the Natural Science Foundation of Jiangsu Province (BK20180489), Young Elite Scientists Sponsorship Program by CAST (2018QNRC001), Fundamental Research Funds for the Central Universities (30918011208), and the National Natural Science Funds for Distinguished Young Scholars (61725402). Z.W. acknowledges the support of the Natural Science Foundation of Shandong Province, China.(ZR2020QE051). B.A.K. and Y.Z. acknowledge funding of this work by the Robert A. Welch Foundation (Grant No. F-1464). H.S. acknowledges the support of Ministry of Education Singapore through the Academic Research Fund under Projects MOE Tier 1, RG 189/17 and RG RG95/19 as well as Tier 2 MOE2016-T2-1-054. H.V.D. and Y.F. gratefully acknowledge TUBA and support in part from NRF-NRFI2016-08 and A*STAR SERC Pharos 52 73 00025. Y.W. thanks the support by the Natural Science Foundation of Jiangsu Province (BK20190446) and NSFC (11904172). J.P.P. and R.E.G. acknowledge the support of Ministerio de Econom{\'i}a, Industria y Competitividad (CTQ2017-82711-P and MDM-2015-0538, partially cofinanced with Fondo Europeo de Desarrollo Regional and Agencia Estatal de Investigaci{\'o}n) and Generalitat Valenciana (IDIFEDER/2018/064 and PROMETEO/2018/138, partially cofinanced with Fondo Europeo de Desarrollo Regional). E.D. and J.H. acknowledge financial support from the Research Foundation—Flanders (FWO Grant Nos. S002019N, G.0B39.15, G.0B49.15, G.0962.13, G098319N, and ZW15_09-GOH6316), the Research Foundation—Flanders postdoctoral fellowships to J.A.S. and E.D. (FWO Grant Nos. 12Y7218N and 12O3719N, respectively), the KU Leuven Research Fund (C14/15/053 and C14/19/079), the Flemish government through long-term structural funding Methusalem (CASAS2, Meth/15/04), the Hercules Foundation (HER/11/14), iBOF funding (PERsist: iBOF-21-085), the Swedish Research Council (VR 2016-04433), Knut and Alice Wallenberg Foundation (KAW 2016.0059), MEXT JSPS Grant-in-Aid for Scientific Research B (19H02550) and Specially Promoted Research (18H05205). R.L.Z.H. acknowledges support from the Royal Academy of Engineering through the Research Fellowship scheme (No. RF\201718\1701) and Downing College Cambridge through the Kim and Juliana Silverman Research Fellowship. M.G. acknowledges a Wenner-Gren fellowship (UPD2017-0223), and L.C. acknowledges a JICA fellowship. A.S. acknowledges the J.C. Bose Fellowship of the Science and Engineering Research Board (SERB). A.L.R. acknowledges the Croucher Foundation of Hong Kong. J.M.L. and Y.Y. acknowledge support from the U.S. Department of Energy, Office of Basic Energy Sciences through the Energy Frontier Research Center, Center for Hybrid Organic Inorganic Semiconductors for Energy (CHOISE). S.K.H. and W.A.T. were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award No. DE-SC0019345. A.L.R. acknowledges the Croucher Foundation of Hong Kong SAR and the Research Grant Council of Hong Kong SAR (GRF 17301520). J.Z.Z. is grateful to financial support from the US NSF (CHE-1904547). A.D. and T.D. acknowledge post-doctoral research fellowship support from Alexander von Humboldt foundation. I.M.-S. acknowledges the financial support from Ministry of Science and Innovation of Spain under Project STABLE (PID2019-107314RB-I00) and Generalitat Valenciana via Prometeo Grant Q-Devices (Prometeo/2018/098). P.V.K. acknowledges the support of the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy, through award (award DE-FC02- 04ER15533). S.D.S. acknowledges the Royal Society and Tata Group (UF150033) and the EPSRC (EP/R023980/1). The work has received funding from the European Research Council under the European Union{\textquoteright}s Horizon 2020 research and innovation programme (HYPERION - grant agreement no. 756962). D.R.G. acknowledges support from the US NSF (DMR-1807394) P.Y, L.N.Q, and M.G. acknowledge the funding from U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-05-CH11231 within the Physical Chemistry of Inorganic Nanostructures Program (KC3103). M.B. acknowledges funding from the Swiss National Science Foundation (Grant No. 200021_192308, “Q-Light - Engineered Quantum Light Sources with Nanocrystal Assemblies”). L.M. acknowledges funding from the FLAG-ERA JTC2019 project PeroGas.",

year = "2021",

month = jun,

day = "17",

doi = "10.1021/acsnano.0c08903",

language = "English (US)",

journal = "ACS Nano",

issn = "1936-0851",

publisher = "American Chemical Society",

}

Dey, A, Ye, J, De, A, Debroye, E, Ha, SK, Bladt, E, Kshirsagar, AS, Wang, Z, Yin, J, Wang, Y, Quan, LN, Yan, F, Gao, M, Li, X, Shamsi, J, Debnath, T, Cao, M, Scheel, MA, Kumar, S, Steele, JA, Gerhard, M, Chouhan, L, Xu, K, Wu, X, Li, Y, Zhang, Y, Dutta, A, Han, C, Vincon, I, Rogach, AL, Nag, A, Samanta, A, Korgel, BA, Shih, C-J, Gamelin, DR, Son, DH, Zeng, H, Zhong, H, Sun, H, Demir, HV, Scheblykin, IG, Mora-Seró, I, Stolarczyk, JK, Zhang, JZ, Feldmann, J, Hofkens, J, Luther, J, Pérez-Prieto, J, Li, L, Manna, L, Bodnarchuk, MI, Kovalenko, MV, Roeffaers, MBJ, Pradhan, N, Mohammed, OF , Bakr, O, Yang, P, Müller-Buschbaum, P, Kamat, PV, Bao, Q, Zhang, Q, Krahne, R, Galian, RE, Stranks, SD, Bals, S, Biju, V, Tisdale, WA, Yan, Y, Hoye, RLZ & Polavarapu, L 2021, 'State of the Art and Prospects for Halide Perovskite Nanocrystals', ACS Nano. https://doi.org/10.1021/acsnano.0c08903

TY - JOUR

T1 - State of the Art and Prospects for Halide Perovskite Nanocrystals

AU - Dey, Amrita

AU - Ye, Junzhi

AU - De, Apurba

AU - Debroye, Elke

AU - Ha, Seung Kyun

AU - Bladt, Eva

AU - Kshirsagar, Anuraj S.

AU - Wang, Ziyu

AU - Yin, Jun

AU - Wang, Yue

AU - Quan, Li Na

AU - Yan, Fei

AU - Gao, Mengyu

AU - Li, Xiaoming

AU - Shamsi, Javad

AU - Debnath, Tushar

AU - Cao, Muhan

AU - Scheel, Manuel A.

AU - Kumar, Sudhir

AU - Steele, Julian A.

AU - Gerhard, Marina

AU - Chouhan, Lata

AU - Xu, Ke

AU - Wu, Xian-gang

AU - Li, Yanxiu

AU - Zhang, Yangning

AU - Dutta, Anirban

AU - Han, Chuang

AU - Vincon, Ilka

AU - Rogach, Andrey L.

AU - Nag, Angshuman

AU - Samanta, Anunay

AU - Korgel, Brian A.

AU - Shih, Chih-Jen

AU - Gamelin, Daniel R.

AU - Son, Dong Hee

AU - Zeng, Haibo

AU - Zhong, Haizheng

AU - Sun, Handong

AU - Demir, Hilmi Volkan

AU - Scheblykin, Ivan G.

AU - Mora-Seró, Iván

AU - Stolarczyk, Jacek K.

AU - Zhang, Jin Z.

AU - Feldmann, Jochen

AU - Hofkens, Johan

AU - Luther, Joseph

AU - Pérez-Prieto, Julia

AU - Li, Liang

AU - Manna, Liberato

AU - Bodnarchuk, Maryna I.

AU - Kovalenko, Maksym V.

AU - Roeffaers, Maarten B. J.

AU - Pradhan, Narayan

AU - Mohammed, Omar F.

AU - Bakr, Osman

AU - Yang, Peidong

AU - Müller-Buschbaum, Peter

AU - Kamat, Prashant V.

AU - Bao, Qialiang

AU - Zhang, Qiao

AU - Krahne, Roman

AU - Galian, Raquel E.

AU - Stranks, Samuel D.

AU - Bals, Sara

AU - Biju, Vasudevanpillai

AU - Tisdale, William A.

AU - Yan, Yong

AU - Hoye, Robert L. Z.

AU - Polavarapu, Lakshminarayana

N1 - KAUST Repository Item: Exported on 2021-06-22 Acknowledgements: L.P. acknowledges support from the Spanish Ministerio de Ciencia e Innovación through Ramón y Cajal grant (RYC2018-026103-I). A.D., T.D., I.V., J.K.S., J.F., M.A.S., P.M.-B. and L.P acknowledge financial support by the Bavarian State Ministry of Science, Research, and Arts through the grant “Solar Technologies go Hybrid (SolTech)” and by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) under Germany’s Excellence Strategy—EXC 2089/1—390776260 (“e-conversion”). J.F., L.P., and V.D acknowledge support by LMU’s “Singapore Initiative” funded within the German Excellence Strategy. H. Zeng acknowledges the support of NSFC (61874054, 51902160), the Natural Science Foundation of Jiangsu Province (BK20180489), Young Elite Scientists Sponsorship Program by CAST (2018QNRC001), Fundamental Research Funds for the Central Universities (30918011208), and the National Natural Science Funds for Distinguished Young Scholars (61725402). Z.W. acknowledges the support of the Natural Science Foundation of Shandong Province, China.(ZR2020QE051). B.A.K. and Y.Z. acknowledge funding of this work by the Robert A. Welch Foundation (Grant No. F-1464). H.S. acknowledges the support of Ministry of Education Singapore through the Academic Research Fund under Projects MOE Tier 1, RG 189/17 and RG RG95/19 as well as Tier 2 MOE2016-T2-1-054. H.V.D. and Y.F. gratefully acknowledge TUBA and support in part from NRF-NRFI2016-08 and A*STAR SERC Pharos 52 73 00025. Y.W. thanks the support by the Natural Science Foundation of Jiangsu Province (BK20190446) and NSFC (11904172). J.P.P. and R.E.G. acknowledge the support of Ministerio de Economía, Industria y Competitividad (CTQ2017-82711-P and MDM-2015-0538, partially cofinanced with Fondo Europeo de Desarrollo Regional and Agencia Estatal de Investigación) and Generalitat Valenciana (IDIFEDER/2018/064 and PROMETEO/2018/138, partially cofinanced with Fondo Europeo de Desarrollo Regional). E.D. and J.H. acknowledge financial support from the Research Foundation—Flanders (FWO Grant Nos. S002019N, G.0B39.15, G.0B49.15, G.0962.13, G098319N, and ZW15_09-GOH6316), the Research Foundation—Flanders postdoctoral fellowships to J.A.S. and E.D. (FWO Grant Nos. 12Y7218N and 12O3719N, respectively), the KU Leuven Research Fund (C14/15/053 and C14/19/079), the Flemish government through long-term structural funding Methusalem (CASAS2, Meth/15/04), the Hercules Foundation (HER/11/14), iBOF funding (PERsist: iBOF-21-085), the Swedish Research Council (VR 2016-04433), Knut and Alice Wallenberg Foundation (KAW 2016.0059), MEXT JSPS Grant-in-Aid for Scientific Research B (19H02550) and Specially Promoted Research (18H05205). R.L.Z.H. acknowledges support from the Royal Academy of Engineering through the Research Fellowship scheme (No. RF\201718\1701) and Downing College Cambridge through the Kim and Juliana Silverman Research Fellowship. M.G. acknowledges a Wenner-Gren fellowship (UPD2017-0223), and L.C. acknowledges a JICA fellowship. A.S. acknowledges the J.C. Bose Fellowship of the Science and Engineering Research Board (SERB). A.L.R. acknowledges the Croucher Foundation of Hong Kong. J.M.L. and Y.Y. acknowledge support from the U.S. Department of Energy, Office of Basic Energy Sciences through the Energy Frontier Research Center, Center for Hybrid Organic Inorganic Semiconductors for Energy (CHOISE). S.K.H. and W.A.T. were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award No. DE-SC0019345. A.L.R. acknowledges the Croucher Foundation of Hong Kong SAR and the Research Grant Council of Hong Kong SAR (GRF 17301520). J.Z.Z. is grateful to financial support from the US NSF (CHE-1904547). A.D. and T.D. acknowledge post-doctoral research fellowship support from Alexander von Humboldt foundation. I.M.-S. acknowledges the financial support from Ministry of Science and Innovation of Spain under Project STABLE (PID2019-107314RB-I00) and Generalitat Valenciana via Prometeo Grant Q-Devices (Prometeo/2018/098). P.V.K. acknowledges the support of the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy, through award (award DE-FC02- 04ER15533). S.D.S. acknowledges the Royal Society and Tata Group (UF150033) and the EPSRC (EP/R023980/1). The work has received funding from the European Research Council under the European Union’s Horizon 2020 research and innovation programme (HYPERION - grant agreement no. 756962). D.R.G. acknowledges support from the US NSF (DMR-1807394) P.Y, L.N.Q, and M.G. acknowledge the funding from U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-05-CH11231 within the Physical Chemistry of Inorganic Nanostructures Program (KC3103). M.B. acknowledges funding from the Swiss National Science Foundation (Grant No. 200021_192308, “Q-Light - Engineered Quantum Light Sources with Nanocrystal Assemblies”). L.M. acknowledges funding from the FLAG-ERA JTC2019 project PeroGas.

PY - 2021/6/17

Y1 - 2021/6/17

N2 - Metal-halide perovskites have rapidly emerged as one of the most promising materials of the 21st century, with many exciting properties and great potential for a broad range of applications, from photovoltaics to optoelectronics and photocatalysis. The ease with which metal-halide perovskites can be synthesized in the form of brightly luminescent colloidal nanocrystals, as well as their tunable and intriguing optical and electronic properties, has attracted researchers from different disciplines of science and technology. In the last few years, there has been a significant progress in the shape-controlled synthesis of perovskite nanocrystals and understanding of their properties and applications. In this comprehensive review, researchers having expertise in different fields (chemistry, physics, and device engineering) of metal-halide perovskite nanocrystals have joined together to provide a state of the art overview and future prospects of metal-halide perovskite nanocrystal research.

AB - Metal-halide perovskites have rapidly emerged as one of the most promising materials of the 21st century, with many exciting properties and great potential for a broad range of applications, from photovoltaics to optoelectronics and photocatalysis. The ease with which metal-halide perovskites can be synthesized in the form of brightly luminescent colloidal nanocrystals, as well as their tunable and intriguing optical and electronic properties, has attracted researchers from different disciplines of science and technology. In the last few years, there has been a significant progress in the shape-controlled synthesis of perovskite nanocrystals and understanding of their properties and applications. In this comprehensive review, researchers having expertise in different fields (chemistry, physics, and device engineering) of metal-halide perovskite nanocrystals have joined together to provide a state of the art overview and future prospects of metal-halide perovskite nanocrystal research.

UR - http://hdl.handle.net/10754/669732

UR - https://pubs.acs.org/doi/10.1021/acsnano.0c08903

U2 - 10.1021/acsnano.0c08903

DO - 10.1021/acsnano.0c08903

M3 - Article

C2 - 34137264

SN - 1936-0851

JO - ACS Nano

JF - ACS Nano

ER -

State of the Art and Prospects for Halide Perovskite Nanocrystals

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