Thermal evolution of the microstructure of nanosized LaFeO3 powders from the thermal decomposition of a heteronuclear complex, La[Fe(CN)6] · 5H2O

Enrico Traversa*, Patrizia Nunziante, Masatomi Sakamoto, Yoshihiko Sadaoka, Maria Cristina Carotta, Giuliano Martinelli

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

61 Scopus citations

Abstract

The thermal decomposition of a heteronuclear complex, La[Fe(CN)6] · 5H2O, leads to the preparation of nanosized single-phase perovskite-type LaFeO3 powders. The microstructural evolution of LaFeO3 with the temperature has been studied by x-ray diffraction (XRD), Fourier transform infrared (FTIR) spectroscopy, scanning electron microscopy (SEM), and transmission electron microscopy (TEM). The product of the decomposition at 500°C consists of nanoporous grains which have the morphology of the complex, but diffracting as a monocrystal of LaFeO3. At the higher temperatures, the nanosized particles start to separate from each other, still keeping the shape of the complex grains and forming soft agglomerates. The formation of LaFeO3 from the complex at low temperatures is facilitated by the formation of an orthorhombic transition phase.

Original languageEnglish (US)
Pages (from-to)1335-1344
Number of pages10
JournalJournal of Materials Research
Volume13
Issue number5
DOIs
StatePublished - May 1998
Externally publishedYes

ASJC Scopus subject areas

  • General Materials Science
  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering

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