Zr-MOF membranes with ultra-fast water-selective permeation towards intensification of esterification reaction

Guozhen Liu; Zhenggang Wang; Cailing Chen; Jiahui Li; Guangyuan Zhou; Wenqi Ji; Gongping Liu; Wanqin Jin

doi:10.1039/d3cc02309e

Zr-MOF membranes with ultra-fast water-selective permeation towards intensification of esterification reaction

Guozhen Liu, Zhenggang Wang, Cailing Chen, Jiahui Li, Guangyuan Zhou, Wenqi Ji, Gongping Liu, Wanqin Jin

Research output: Contribution to journal › Article › peer-review

9 Scopus citations

Abstract

Well-intergrown polycrystalline UiO-66 membranes were successfully synthesized on polymeric substrate under mild synthesis conditions of low temperature and short synthesis time. Benefiting from angstrom-sized lattice apertures, the UiO-66 membranes with fast water selective transport channels revealed an unprecedented high solvents dehydration performance with permeation flux of up to ~6100 g·m-2·h-1 and separation factor of ~7500, showing great potential for intensification of esterification reaction.

Original language	English (US)
Journal	CHEMICAL COMMUNICATIONS
DOIs	https://doi.org/10.1039/d3cc02309e
State	Published - May 31 2023

ASJC Scopus subject areas

Materials Chemistry
Surfaces, Coatings and Films
Metals and Alloys
Ceramics and Composites
General Chemistry
Catalysis
Electronic, Optical and Magnetic Materials

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10.1039/d3cc02309e

https://repository.kaust.edu.sa/bitstream/10754/692380/1/d3cc02309e_removed.pdf

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title = "Zr-MOF membranes with ultra-fast water-selective permeation towards intensification of esterification reaction",

abstract = "Well-intergrown polycrystalline UiO-66 membranes were successfully synthesized on polymeric substrate under mild synthesis conditions of low temperature and short synthesis time. Benefiting from angstrom-sized lattice apertures, the UiO-66 membranes with fast water selective transport channels revealed an unprecedented high solvents dehydration performance with permeation flux of up to ~6100 g·m-2·h-1 and separation factor of ~7500, showing great potential for intensification of esterification reaction.",

author = "Guozhen Liu and Zhenggang Wang and Cailing Chen and Jiahui Li and Guangyuan Zhou and Wenqi Ji and Gongping Liu and Wanqin Jin",

note = "KAUST Repository Item: Exported on 2023-06-06 Acknowledgements: This work was supported by the Natural Science Foundation of Jiangsu Province (BK20220002), the National Natural Science Foundation of China (22278210, 22038006) and the China Postdoctoral Science Foundation (2022TQ0147, 2022M721584).",

year = "2023",

month = may,

day = "31",

doi = "10.1039/d3cc02309e",

language = "English (US)",

journal = "CHEMICAL COMMUNICATIONS",

issn = "1359-7345",

publisher = "ROYAL SOC CHEMISTRY",

}

TY - JOUR

T1 - Zr-MOF membranes with ultra-fast water-selective permeation towards intensification of esterification reaction

AU - Liu, Guozhen

AU - Wang, Zhenggang

AU - Chen, Cailing

AU - Li, Jiahui

AU - Zhou, Guangyuan

AU - Ji, Wenqi

AU - Liu, Gongping

AU - Jin, Wanqin

N1 - KAUST Repository Item: Exported on 2023-06-06 Acknowledgements: This work was supported by the Natural Science Foundation of Jiangsu Province (BK20220002), the National Natural Science Foundation of China (22278210, 22038006) and the China Postdoctoral Science Foundation (2022TQ0147, 2022M721584).

PY - 2023/5/31

Y1 - 2023/5/31

N2 - Well-intergrown polycrystalline UiO-66 membranes were successfully synthesized on polymeric substrate under mild synthesis conditions of low temperature and short synthesis time. Benefiting from angstrom-sized lattice apertures, the UiO-66 membranes with fast water selective transport channels revealed an unprecedented high solvents dehydration performance with permeation flux of up to ~6100 g·m-2·h-1 and separation factor of ~7500, showing great potential for intensification of esterification reaction.

AB - Well-intergrown polycrystalline UiO-66 membranes were successfully synthesized on polymeric substrate under mild synthesis conditions of low temperature and short synthesis time. Benefiting from angstrom-sized lattice apertures, the UiO-66 membranes with fast water selective transport channels revealed an unprecedented high solvents dehydration performance with permeation flux of up to ~6100 g·m-2·h-1 and separation factor of ~7500, showing great potential for intensification of esterification reaction.

UR - http://hdl.handle.net/10754/692380

UR - http://pubs.rsc.org/en/Content/ArticleLanding/2023/CC/D3CC02309E

U2 - 10.1039/d3cc02309e

DO - 10.1039/d3cc02309e

M3 - Article

C2 - 37288520

SN - 1359-7345

JO - CHEMICAL COMMUNICATIONS

JF - CHEMICAL COMMUNICATIONS

ER -

Zr-MOF membranes with ultra-fast water-selective permeation towards intensification of esterification reaction

Abstract

ASJC Scopus subject areas

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